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the claim
Reactions between species with different total electron spin multiplicities are spin-forbidden
the verdict
SUPPORTED
the evidence backs this
refutedsupported
the weight of evidence
3 sources for · 0 against

Chemical reactions and transitions between species possessing different total electron spin multiplicities are fundamentally spin-forbidden, requiring mechanisms such as spin-orbit coupling or intersystem crossing to proceed.

Evidence for · 3
2025 · cited by 3
The paper discusses spin crossings between electronic states with different spin multiplicities, such as singlet and triplet, which require nonadiabatic or spin-orbit coupling.
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The analysis

The retrieved literature consistently supports the fundamental premise in quantum chemistry and reaction dynamics that reactions or transitions involving a change in total electron spin multiplicity (e.g., between singlet and triplet states) are spin-forbidden and typically necessitate spin-orbit coupling or intersystem crossing to occur.

More for · 2
2026 · cited by 0
The study notes that spin-orbit coupling enables spin-forbidden release of triplet oxygen in atom-transfer channels during reactions.
2026 · cited by 0
The paper examines reactions between ionic and neutral species where exothermic product channels require an intersystem crossing due to differing spin multiplicities.
Everything we examined (12)
  1. Roadmap for Molecular Benchmarks in Nonadiabatic Dynamics.peer-reviewedno side takennot shown: read and judged not to bear on this claim
  2. Performance of quantum chemistry methods for a benchmark set of spin-state energetics derived from experimental data of 17 transition metal complexes (SSE17).peer-reviewedno side takennot shown: read and judged not to bear on this claim
  3. COLUMBUS─An Efficient and General Program Package for Ground and Excited State Computations Including Spin-Orbit Couplings and Dynamics.peer-reviewedno side takennot shown: read and judged not to bear on this claim
  4. AIMNet2-NSE: A Transferable Reactive Neural Network Potential for Open-Shell Chemistry.peer-reviewedno side takennot shown: read and judged not to bear on this claim
  5. Organic Spin-State Photoswitches.peer-reviewedno side takennot shown: read and judged not to bear on this claim
  6. Noncollinear Spin-Flip TDDFT for Potential Energy Surface Crossings: Conical Intersections and Spin Crossings.peer-reviewedsupports
  7. High-resolution spectroscopy of [H,C,N]&lt;sup&gt;+&lt;/sup&gt;: III. Infrared Ã&lt;sup&gt;2&lt;/sup&gt;Σ&lt;sup&gt;+&lt;/sup&gt; ← X̃&lt;sup&gt;2&lt;/sup&gt;Π electronic transition of HCN<sup/>.peer-reviewedno side takennot shown: read and judged not to bear on this claim
  8. Quantum suppression of cold reactions far from the s-wave energy limit.peer-reviewedno side takennot shown: read and judged not to bear on this claim
  9. Electron transfer drives hydroxyl radical formation in peroxone reactions.peer-reviewedsupports
  10. Aromaticity-Induced Spin State Switching and High-Spin States in Non-Alternant Polyradicals.peer-reviewedno side takennot shown: read and judged not to bear on this claim
  11. Kinetics of Submerged Intersystem Crossings in Strongly Coupled Ion-Molecule Reactions: I&lt;sup&gt;+&lt;/sup&gt; + CH&lt;sub&gt;3&lt;/sub&gt;X (X = F, Cl, Br, I).peer-reviewedsupports
  12. Interface-Confined Triplet Sensitization and Photon Upconversion in Pyrene-Tetracyanobenzene Charge-Transfer Cocrystals.peer-reviewedno side takennot shown: read and judged not to bear on this claim
The paper trail · every fact has a biography
first checked05 Aug 2026
judged → SUPPORTED · 7905 Aug 2026
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